Additionally, ether-based and liquefied gas electrolytes with weak solvation, high Li affinity and superior ionic conductivity are promising candidates for Li metal batteries working at ultralow temperature.
The Li stabilizing strategies including artificial SEI, alloying, and current collector/host modification are promising for application in the low-temperature batteries. However, expeditions on such aspects are presently limited, with numerous efforts being devoted to electrolyte designs. 3.3.1. Interfacial regulation and alloying
All in all, to achieve the high capacity retention, long lifespan, and high mass/volume energy density of LMBs at low temperature, more efforts and expeditions should be conducted, concurrently considering the ion transport and mass/electron transfer within the cathode, anode and their interfaces in addition to the bulk electrolyte.
Li et al. reported that LMO/Li battery still has a high Li + diffusion coefficient of 10–12 cm 2 s -1 at −20 °C compared to that of room temperature (10 –10 cm 2 s -1) . However, LMO delivers higher R ct than LFP and LCO at various low temperature.
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